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In the absence of doping, interface dipoles and other interfacial effects and assuming vacuum level alignment the energy barrier for charge carrier injection is in first approximation given by the energetic offset between the work functions of the used metals and the energy levels of the organic material. A review of the synthesis, structure, and properties of metal–organic frameworks (MOFs) is presented, highlighting the important advances in their research over the past decade. CRYSTALS is a software package for single crystal X-ray structure refinement and analysis. The download contains CRYSTALS, Cameron and specially recompiled versions of SIR92 and SHELXS.There are also transparent links to SUPERFLIP (Lucas Palatinus’s structure solution by charge flipping), MCE (a Fourier map and voids viewer by Rohlicek & Husak) both of which are distributed with CRYSTALS. 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